PULSED LASER DEPOSITION OF NOVEL SPINEL MATERIALS FOR PHOTOVOLTAIC CONVERSION

1,2 HOLOVSKÝ Jakub
Co-authors:
1,2 LANDOVÁ Lucie 3 HORÁK Lukáš 3 DOPITA Milan 1 JAIN Naini 1 HORYNOVÁ Eva 1,2 NEYKOVA Neda 2 LIBERTÍNOVÁ Jitka 1 SHARMA Rupendra Kumar
Institutions:
1 Centre for Advanced Photovoltaics, Faculty of Electrical Engineering, Czech Technical University in Prague, Prague, Czech Republic, EU, jakub.holovsky@fel.cvut.cz
2 Institute of Physics, Czech Academy of Sciences, Prague, Czech Republic, EU
3 Faculty of Mathematics and Physics, Charles University, Prague, Czech Republic, EU
Conference:
16th International Conference on Nanomaterials - Research & Application, OREA Congress Hotel Brno, Czech Republic, EU, October 16 - 18, 2024
Proceedings:
Proceedings 16th International Conference on Nanomaterials - Research & Application
Pages:
177-181
ISBN:
978-80-88365-24-2
ISSN:
2694-930X
Published:
28th February 2025
Metrics:
32 views / 16 downloads
Abstract

While all traditional photovoltaic materials are covalent compounds with coordination number 4, currently the most progressive materials - hybrid halide perovskites - have coordination number 6 and are ionic. This can be the key to success, especially regarding surface electronic properties, which are essential for polycrystalline semiconductors. This motivates us to explore completely new materials - cubic lithium thiospinels - and compare them with the former. Li thiospinels are prepared from stoichiometrically mixed precursors as a pellet in a nitrogen-filled glovebox. This tablet serves as a target in Pulsed Laser Deposition (PLD) and a special chamber is constructed that avoids air exposure of the precursor tablet during the loading. Thin films of lithium thiospinels are deposited on glass substrates and they are characterized by X-ray diffraction and optically by Photothermal Deflection Spectroscopy for accurate determination of absorption edge. Results are promising and demonstrate the validity of this approach.

Keywords: Thiospinels, methodology, hybrid halide perovskites, novel material, pulsed laser deposition

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