ADVANCED PREPARATION AND CHARACTERIZATION OF PEDOT-BASED NONWOVEN MATERIALS FOR WEARABLE ELECTRONICS

1 SLEJKO Emanuele Alberto
Co-authors:
1 CARRARO Giovanni 2 CAVALLO Dario 2 SPOTORNO Roberto 1 SMERIERI Marco
Institutions:
1 CNR-IMEM – Institute of Materials for Electronics and Magnetism, National Research Council of Italy, Genoa, Italy, EU
2 Department of Chemistry, University of Genoa, Genoa, Italy, EU
Conference:
16th International Conference on Nanomaterials - Research & Application, OREA Congress Hotel Brno, Czech Republic, EU, October 16 - 18, 2024
Proceedings:
Proceedings 16th International Conference on Nanomaterials - Research & Application
Pages:
278-283
ISBN:
978-80-88365-24-2
ISSN:
2694-930X
Published:
28th February 2025
Metrics:
30 views / 14 downloads
Abstract

Poly(3,4-ethylenedioxythiophene)-polystyrene sulfonate (PEDOT-PSS) nanofiber-based materials represent advanced solutions for application in wearable electronics due to their biocompatibility, lightweight, permeability and improved sensitivity related to their large surface area. Since PEDOT is a conductive polymer, the electrospinning process for manufacturing thin, flexible nonwovens made of homogeneous nanofibers is not well-studied yet. In this research, we have investigated the fabrication and characterization of electrospun conductive nanofibers composed of varying concentrations of PEDOT-PSS mixed with poly(ethylene oxide) (PEO). The electrospinning technique was employed to produce these conductive nonwovens, and their morphological properties were evaluated using scanning electron microscopy (SEM). To enhance the water resistance of nanofibers, a thermal treatment was applied to remove excess PEO. The resulting samples demonstrated significant improvements in water stability, whereas untreated samples dissolved in pure water almost immediately. Electrical characterization of conductive nonwovens was performed, revealing resistivity in several hundreds of Ohm•m. To further investigate the electrical response and electrochemical behavior of the material when in contact with specific compounds, we conducted electric impedance spectroscopy (EIS) and cyclic voltammetry (CV). The EIS measurements provided insights into the impedance characteristics, while the CV analysis highlighted the occurrence of reversible faradaic reactions. Our findings suggest that the optimized PEDOT-PSS/PEO nanofibers exhibit promising electrical and electrochemical properties, making them suitable for applications in flexible electronics and wearable sensors. This study contributes to the understanding of the relationship between the fabrication process, structural morphology, and functional performance of electrospun conductive nonwovens with the potential to significantly impact the wearable technology field.

Keywords: Nonwovens, conductive polymers, electrospinning, flexible electronics

© This is an open access article distributed under the Creative Commons Attribution License which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.

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