DIMINISHING OF STEEL CORROSION IN ACID ENVIRONMENT USING THIN BI-LAYER SURFACES OF MONO-CARBOXYL-SUBSTITUTED A3B PORPHYRIN AND MNTA2O6

1 BIRDEANU Mihaela
Co-authors:
2 BIRDEANU Aurel-Valentin 3 FRATILESCU Ion 3 FAGADAR-COSMA Eugenia
Institutions:
1 National Institute for Research and Development in Electrochemistry and Condensed Matter, Timisoara, Romania, mihaelabirdeanu@gamil.com
2 National Research & Development Institute for Welding and Material Testing - ISIM, Timisoara, Romania, valentinbirdeanu@yahoo.com
3 Institute of Chemistry “Coriolan Dragulescu”, Timisoara, Romania, efagadar@yahoo.comion.fratilescu@gmail.com
Conference:
13th International Conference on Nanomaterials - Research & Application, Orea Congress Hotel Brno, Czech Republic, EU, October 20 - 22, 2021
Proceedings:
Proceedings 13th International Conference on Nanomaterials - Research & Application
Pages:
448-453
ISBN:
978-80-88365-00-6
ISSN:
2694-930X
Published:
22nd November 2021
Proceedings of the conference were published in Scopus.
Metrics:
475 views / 298 downloads
Abstract

It is already known, that porphyrin–bases are offering better protection against steel corrosion than metalloporphyrins due to their ability to form very stable metallic complexes by linking in their inner core the iron contained in different steels. In this respect, 5-(4-carboxy-phenyl)-10,15,20-tris-(4-phenoxy-phenyl)-porphyrin was synthesized by multicomponent Adler-Longo synthesis, using two different aldehydes and pyrrole, characterized to certify the structure and further used for formulating double thin layers in all possible combinations with MnTa2O6. The pseudo-binary oxide nanomaterials MnTa2O6 were synthesized by solid-state method. The corrosion protection exhibited by these nanostructures alone or in composites after deposition on carbon steel was comparatively assessed in acid environment. Different electrochemical techniques, such as: open circuit potential measurement and potentiodynamic polarization technique with Tafel representation were used. The performed tests reveal that corrosion protection is fairly good, with the best results indicating that the electrode covered with 5-(4-carboxy-phenyl)-10,15,20-tris-(4-phenoxy-phenyl)-porphyrin / MnTa2O6 has offered the best corrosion inhibition efficiency of 86.05

Keywords: Mono-carboxyl-substituted A3B porphyrins, MnTa2O6, steel, corrosion inhibition, Tafel curves

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