INFLUENCE OF ISOTHERMAL EXPOSURE ON MICROSTRUCTURAL CHANGES RESULTING IN DELAMINATION OF EUTECTIC AL2O3+ZRO2+SIO2 THERMAL BARRIER COATINGS

1,2 JECH David
Co-authors:
1,2 ČELKO Ladislav 3 CHRÁSKA Tomáš 1,2 SLÁMEČKA Karel 1,2 KLAKURKOVÁ Lenka 3 DUBSKÝ Jiří 1,2 ŠVEJCAR Jiří
Institutions:
1 Brno University of Technology (BUT), Central European Institute of Technology (CEITEC), Research Group of Advanced Coatings, Brno, Czech Republic, EU, david.jech@ceitec.vutbr.cz
2 Brno University of Technology (BUT), Faculty of Mechanical Engineering, Institute of Materials Science and Engineering, Brno, Czech Republic, EU, jechdavid@gmail.com
3 Institute of Plasma Physics, Academy of Sciences of the Czech Republic, Prague, Czech Republic, EU david.jech@ceitec.vutbr.cz, ladislav.celko@ceitec.vutbr.cz, tchraska@ipp.cas.cz, karel.slamecka@ceitec.vutbr.cz, lenka.klakurkova@ceitec.vutbr.cz, dubsky@ipp.cas.cz, jiri.svejcar@ceitec.vutbr.cz
Conference:
23rd International Conference on Metallurgy and Materials, Hotel Voronez I, Brno, Czech Republic, EU, May 21 - 23, 2014
Proceedings:
Proceedings 23rd International Conference on Metallurgy and Materials
Pages:
885-889
ISBN:
978-80-87294-52-9
ISSN:
2694-9296
Published:
18th June 2014
Proceedings of the conference were published in Web of Science and Scopus.
Metrics:
270 views / 145 downloads
Abstract

Eutectic ceramic Al2O3-ZrO2-SiO2 also termed Eucor (as a top coat) and CoNiCrAlY (as a bond coat) coatings were sprayed onto the surface of recently developed fine-grained cast polycrystalline nickel-based superalloy Inconel 713 LC by means of water stabilized plasma (WSP) and atmospheric plasma spraying (APS) techniques, respectively. Specimens were subjected to isothermal oxidation at 1050 °C for 10, 50, 100, 200 and 500 hours in ambient atmosphere, prior to which a half of the as-sprayed specimens was annealed at the temperature of 950 °C for 10 hours. Influence of short-time and long-time isothermal exposure on interactions at the bond-coat/top-coat interface was studied. The uniform and continuous oxide layer, also termed the thermally grown oxide (TGO), was formed and grew at the bond-coat/top-coat interface in all samples, both with and without the heat pre-treatment. Relationship between the dwell time, heat treatment and TGO growth kinetics was quantified. Microstructural changes at top-coat/bond-coat interface were investigated by means of a scanning electron microscope equipped with an energy dispersive microanalyzer and by means of image analysis techniques. Delamination of the ceramic top coat in the region near to the top-coat/TGO interface was evocated by stresses initiated in the Eucor top coat due to its shrinkage during cooling.

Keywords: Thermal Barrier Coatings, Atmospheric Plasma Spraying, Isothermal heat treatment, Electron microscopy, Image analysis

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